Makio Inoue

Captain Harlock / Phantom F. Harlock II

Kei Tomiyama

Tochirô Ôyama

Yūjirō Ishihara

Phantom F. Harlock I

Shuichi Ikeda

Zoll

Eiko Masuyama

The Witch

Shūichirō Moriyama

Old Tokargan Soldier

Reiko Tajima

Queen Emeraldas

Hiromi Tsuru

Mira

Yuriko Yamamoto

La Mîmé

Takeshi Aono

Murigson

Hidekatsu Shibata

Black-Suited Commander (voice)

Reiko Mutoh

Maya (voice)

Tarō Ishida

Zeda (voice)

Koji Yada

Illumidas Officer